Jpn. J. Appl. Phys. 43 (2004) pp. L1436-L1438 |Previous Article| |Next Article| |Table of Contents|
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Letter
Clathrate-like Ordering in Liquid Water Induced by Infrared Irradiation
Tetsuro Yokono1,
Shigezo Shimokawa1,2,,
Tadahiko Mizuno3,
Makio Yokono3 and
Toshio Yokokawa4
1Techno-Science Laboratory, 22-18 Nakamachi, Oasa, Ebetsu 069-0854, Japan
2Center for Advanced Science and Technology, Hokkaido University, Kita-ku Kita-21 Nishi-11, Sapporo 001-0021, Japan
3Graduate School of Engineering, Hokkaido University, Kita-ku Kita-12 Nishi-8, Sapporo 060-8628, Japan
4Faculty of Science, Hokkaido University, Kita-ku Kita-10 Nishi-8, Sapporo 060-8628, Japan
(Received June 18, 2004; accepted August 27, 2004; published October 15, 2004)
X-ray diffraction experiments revealed that when liquid water is exposed to infrared irradiation a solidlike ordering of water molecules is induced. The ordered structure was found to be either of the clathrate hydrates I and II or their mixture. It takes more than 24 h for the ordered structure to return to the original state, as long as it is kept below 278 K.
KEYWORDS:
X-ray diffraction, liquid water, cooperative propagation, infrared irradiation, clathrate hydrate, solidlike ordering
URL:
http://jjap.ipap.jp/link?JJAP/43/L1436/
DOI: 10.1143/JJAP.43.L1436
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